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- W2035714887 abstract "Calculations using a Lennard-Jones type 9-3 potential are carried out for As4 molecules physisorbed on an arsenic crystal surface to elucidate factors determining the extent to which gaseous and evaporating molecules achieve equilibrium with the surface. Equilibrium residence lifetimes for adsorbed molecules are calculated for values of the depth of the potential well between the molecule and the surface of 2.5 to 15 kcalmole. The fraction of molecules achieving equilibrium during free vaporization is calculated for various values of the molecule-surface potential well depth (2.5–15 kcalmole), initial energy of the molecules perpendicular to the surface (0.25–15 kcalmole), and the fraction of energy lost per vibrational collision with the surface (0.01–0.5). For the values of these parameters most likely to apply to arsenic, the computations imply that some detectable fraction of evaporating As4 molecules may leave the surface thermally excited, but that a significant fraction attains equilibrium." @default.
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- W2035714887 date "1972-02-01" @default.
- W2035714887 modified "2023-09-26" @default.
- W2035714887 title "Factors determining residence lifetimes of As4 molecules on an arsenic (111) surface" @default.
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- W2035714887 doi "https://doi.org/10.1016/0039-6028(72)90237-3" @default.
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