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• W2035735513 abstract "The structure of supported metal catalysts can often be related to the fraction of the total atoms which is exposed on the surface (FE). The catalytic property related to the structure is the turnover frequency (TOF), the rate per unit of surface atoms. The particular behavior of these atoms can then be expressed via their Taylor ratio, a function of the way the surface atoms form an active site. For particles of FE < 0.5, it is interesting to relate the Taylor ratio to the geometry of idealized crystallites. The relation between Taylor ratio and FE is presented graphically for some ideal crystallites, based on several possible geometrically defined active sites. Some experimental data can be explained by the analysis, but there are many exceptions. Although a graph of log TOF against log FE may sometimes produce a straight line, there is no reason to expect such a relation to be valid in general." @default.
• W2035735513 created "2016-06-24" @default.
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• W2035735513 date "1989-12-01" @default.
• W2035735513 modified "2023-10-11" @default.
• W2035735513 title "Some geometric aspects of structure sensitivity" @default.
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• W2035735513 doi "https://doi.org/10.1016/0021-9517(89)90270-4" @default.
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