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• W2035861957 startingPage "13773" @default.
• W2035861957 abstract "We have measured the scattering-angle dependence of the Raman intensity of the ring breathing mode (1005 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$) of pyridine molecules adsorbed on silver electrodes with rough surfaces. For both large and small surface roughness (rms amplitude ensuremath{sim}2500 and ensuremath{sim}90 AA{}, respectively), the Raman intensity decreases monotonically with increasing scattering angles measured from the surface normal. The depolarization ratio shows weak angular dependence within the range between 0.5 and 1.3. The observed angular dependence and depolarization ratio of Raman intensity cannot be explained by the electromagnetic theory that treats interface roughness as a perturbation. Thus we have adopted an effective dielectric-layer model to obtain a better agreement with the experimental data. In this model the scattering dipoles are embedded in an effective dielectric layer formed by oxidation-reduction cycles of the electrode surface." @default.
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• W2035861957 date "1993-05-15" @default.
• W2035861957 modified "2023-09-27" @default.
• W2035861957 title "Scattering-angle dependence of the Raman intensity of pyridine molecules adsorbed on rough silver electrodes" @default.
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• W2035861957 doi "https://doi.org/10.1103/physrevb.47.13773" @default.
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