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- W2035877055 abstract "The initial kinetics of the dissolution of vitreous silica was measured in aqueous solutions as a function of pH (5–11) and ionic content ((Na,Mg) Clx:0.1–3.5 M) at 25°C. The apparent rate constant of silica dissolution, k1, increased by a factor of 360 from pH 5 to pH 11 at NaCl = 0.70 M. The addition of Mg2+ to NaCl solutions, where the total ionic strength was maintained constant, had no effect on k1 at pH 8 but k1 decreased by about 30% at pH 9 (Mg2+ = 0.055 M). In NaCl solutions, k1 is shown to be an explicit function of surface charge. A plot of log10 (dissolution rate) vs log10 (surface charge) is linear at lower surface charge with a slope of 1.94, suggesting that two surface excess OH−'s are in the transition state of the rate-determining step of silica dissolution." @default.
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- W2035877055 title "The initial kinetics of the dissolution of vitreous silica in aqueous media" @default.
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- W2035877055 doi "https://doi.org/10.1016/0021-9797(79)90307-2" @default.
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