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• W2035888712 abstract "Atomic-scale structure studies involving synchrotron x-ray diffraction (SXRD) and pair distribution function (PDF) analysis on a series of YMnO${}_{3}$ particles with sizes ranging from 467 $ifmmodepmelsetextpmfi{}$ 42 (bulk) to 10 $ifmmodepmelsetextpmfi{}$ 1 nm are presented. Studies reveal that while the nanoparticles retain most of the characteristics of the layered hexagonal-type structure of the bulk, substantial local atomic displacements arise with diminishing particle size. The displacements lead to a very substantial loss of structural coherence in the particles of size smaller than 100 nm. The displacements mostly affect the yttrium (Y) atoms and to a lesser extent the Mn-O sublattice in YMnO${}_{3}$. We argue that the increased displacement of Y atoms along the polar $c$ axis of the hexagonal unit cell may result in enhanced local ferroelectric distortions with decreasing particle size. The planar, that is, $a$- and $b$-axis direction displacements of Y atoms, however, may interfere with the cooperative ferroelectricity of nanosized YMnO${}_{3}$, so future efforts to employ YMnO${}_{3}$ in nanoscale applications should take them into account." @default.
• W2035888712 created "2016-06-24" @default.
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• W2035888712 date "2012-09-04" @default.
• W2035888712 modified "2023-10-16" @default.
• W2035888712 title "Structural coherence and ferroelectric order in nanosized multiferroic YMnO<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>3</mml:mn></mml:msub></mml:math>" @default.
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• W2035888712 doi "https://doi.org/10.1103/physrevb.86.094101" @default.
• W2035888712 hasPublicationYear "2012" @default.
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