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- W2036334304 abstract "Raman scattering measurements have been carried out on poly(propylene glycol) complexed with LiCF3SO3 salt over a wide salt concentration range, the ether oxygen to alkali metal cation ratios (O:M) ranging from 4820: 1 to 12: 1. The relative concentrations of solvated anions, anion-cation pairs and ionic aggregates have been calculated from an analysis of the symmetric anion stretch. The degree of association is found to be almost constant in the O:M range 4820: 1–40: 1 whereafter it increases with increasing salt concentration. The results show that the dramatic increase reported for the molar conductivity in the O:M range 1000:1–40: 1 cannot be explained by the redissociation of contact ion pairs or the formation of conducting triplets. Instead the major contribution to the conductivity increase seems to be a concentration dependent enhancement of the ionic mobility. A percolation based ionic hopping process involving exchange between ions in pairs and dissolved ions, either free or coordinated to ether oxygen sites, is advanced as a possible microscopic mechanism." @default.
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- W2036334304 date "1995-10-01" @default.
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- W2036334304 title "The molar conductivity behavior in polymer electrolytes at low salt concentrations; A Raman study of poly(propylene glycol) complexed with LiCF3SO3" @default.
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- W2036334304 doi "https://doi.org/10.1016/0013-4686(95)00196-l" @default.
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