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• W2036388374 startingPage "3112" @default.
• W2036388374 abstract "Recent demonstrations in doped semiconductor nanocrystals establish that a plasmon resonance can be sustained by a handful of charge carriers, much smaller in number than conventionally thought. This finding raises questions about the physical nature of such a collective resonance, a fundamental question in condensed matter and many-body physics, which the author addresses here by means of a plasmon-in-a-box model. A small number of carriers confined within a nanocrystal exhibit multiple transitions of individual carriers between quantized states. However, as carriers are progressively added, spectral lines associated with single-carrier excitations evolve into a band representing a collective resonance. This evolution is gradual, and it involves an intermediate regime where single-carrier excitations and few-carrier collective excitations coexist, until, at high carrier numbers, a purely classical collective resonance involving all carriers in the nanocrystal is sustained. The author finds that the emergence of the plasmon resonance is a density-driven transition; at high enough carrier densities, the Coulomb repulsion between carriers becomes strong enough to allow individual carriers to overcome their confinement to the nanocrystal lattice and to participate in a collective excitation within the mean Coulomb field of other carriers. The findings represent deeper insight into the physical picture of a plasmon resonance and serve as a potential design guide for nanoscale optoelectronic components and photocatalytic plasmonic clusters." @default.
• W2036388374 created "2016-06-24" @default.
• W2036388374 creator A5030902865 @default.
• W2036388374 date "2014-08-29" @default.
• W2036388374 modified "2023-09-27" @default.
• W2036388374 title "Plasmon-in-a-Box: On the Physical Nature of Few-Carrier Plasmon Resonances" @default.
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• W2036388374 doi "https://doi.org/10.1021/jz501456t" @default.
• W2036388374 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26276321" @default.
• W2036388374 hasPublicationYear "2014" @default.
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