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- W2036582307 abstract "In this work we use a new approach to investigate the equilibrium and linear dynamic-mechanical response of a polymer network. The classical Rouse model is extended to incorporate quenched constraints on its end-boundary conditions; a microscopic stress tensor for the network system is then derived in the affine deformation limit. To test the model we calculate the macroscopic stress in equilibrium, corresponding to the long-time limit of relaxation. Particular attention is paid to the treatment of compressibility and hydrostatic pressure in a sample with open boundaries. Although quite different in general, for small strains the model compares well with the classic equilibrium rubber-elasticity models. The dynamic shear modulus is obtained for a network relaxing after an instantaneous step strain by keeping track of relaxation of consecutive Rouse modes of constrained network strands. The results naturally cover the whole time range--from the dynamic glassy state down to the equilibrium incompressible rubber plateau." @default.
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- W2036582307 date "2005-07-15" @default.
- W2036582307 modified "2023-10-11" @default.
- W2036582307 title "Constrained Rouse model of rubber viscoelasticity" @default.
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- W2036582307 doi "https://doi.org/10.1063/1.1955445" @default.
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