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• W2036693093 abstract "Abstract This study explored the possibility of using waste organic solvent as the source of volatile organic compound (VOC) and it served as a reducing agent of selective catalytic reduction (SCR) deNO x process, in which the VOC itself can be catalytically oxidized on the mesoporous Cu and/or Al substituted MCM-41 catalysts. The synthesized Cu–Al–MCM-41 catalysts were extensively characterized by powder low-angle X-ray diffraction (XRD), N 2 adsorption–desorption measurements, transmission electron microscopy (TEM), UV–Visible diffuse reflectance spectroscopy (UV–Vis DRS), 27 Al magic angle spinning-nuclear magnetic resonance spectroscopy (MAS-NMR), electron paramagnetic resonance spectroscopy (EPR) and inductively coupled plasma–mass spectrometer (ICP–MS) analysis. The XRD, TEM and N 2 adsorption–desorption studies clearly demonstrated the presence of a well ordered long range hexagonal array with uniform mesostructures. The Cu–Al–MCM-41 materials showed a better long-term-stability than that of copper ion-exchanged H–ZSM-5 (Cu–ZSM-5) zeolite. The Cu–Al–MCM-41 material was found to be an efficient catalyst than that of Cu–MCM-41 without aluminum for the simultaneous catalytic abatement of NO x and VOCs, which was attributed to the presence of well dispersed and isolated Cu 2+ ions on the Cu–Al–MCM-41 catalyst as observed by UV–Vis DRS and EPR spectroscopic studies. And the presence of aluminum (Al 3+ ions) within the framework of Cu–Al–MCM-41 stabilized the isolated Cu 2+ ions thus it led to higher and stabilized activity in terms of NO x reduction." @default.
• W2036693093 created "2016-06-24" @default.
• W2036693093 creator A5046923126 @default.
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• W2036693093 date "2009-01-01" @default.
• W2036693093 modified "2023-10-16" @default.
• W2036693093 title "Bifunctional mesoporous Cu–Al–MCM-41 materials for the simultaneous catalytic abatement of NOx and VOCs" @default.
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• W2036693093 doi "https://doi.org/10.1016/j.micromeso.2008.06.016" @default.
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