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• W2036702316 endingPage "572" @default.
• W2036702316 startingPage "563" @default.
• W2036702316 abstract "Recent work with binary blends of narrow-distribution polystyrenes has shown that the elastic properties depend on the molecular weight distribution in a complex way when the molecular weights are both above the entanglement point. In particular the steady-state compliance Je0 becomes proportional to w2−2 when w2, the weight fraction of the higher molecular-weight species, approaches unity. These results led to the suggestion that a high-order (nonlinear) blending law might be required above the entanglement point.In the present work the general problem of modelling the molecular weight dependence in the transition, rubbery plateau, and terminal flow regimes is discussed, including models for the juncture points between these regions. A general mathematical framework is presented which includes the Rouse spectrum and a linear blending law for low molecular weights (and also for the short-time portion of the spectrum generally); a network spectrum and a quadratic blending law for the higher molecular weights; and a mixture of these models for intermediate cases. Also, results for wide-distribution mixtures and for n-th order blending laws are stated." @default.
• W2036702316 created "2016-06-24" @default.
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• W2036702316 date "1970-09-01" @default.
• W2036702316 modified "2023-09-23" @default.
• W2036702316 title "A Constitutive Model for Molecular Weight and Concentration Effects in Polymer Blends" @default.
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• W2036702316 doi "https://doi.org/10.1295/polymj.1.563" @default.
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