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• W2036706219 abstract "Upon photolysis of solid CO2 by 1216-Å radiation, very high yields of CO3 have been obtained. There is no evidence for the production of hydrogen-containing species in experiments in which photolytically produced H or D atoms are also present. Experimental evidence supports a C2υ structure for CO3 in its ground state, as predicted by molecular orbital calculations. The vibrational frequency pattern for the planar modes of isotopically substituted species of CO3 has been fitted to a valence force potential having a minimal number of interaction force constants, assuming both an open structure having an O–C–O angle of 80° and a three-membered ring structure having an O–C–O angle of 65°. Although the force constants obtained for the ring structure appear to be quite reasonable, exceptionally large values have been obtained for the O–C–O bending force constant and for all of the interaction constants for the open structure. On this basis, the three-membered ring structure is favored for CO3 in its ground state." @default.
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• W2036706219 date "1971-02-01" @default.
• W2036706219 modified "2023-10-14" @default.
• W2036706219 title "Infrared Spectrum and Structure of the Species CO3" @default.
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• W2036706219 doi "https://doi.org/10.1063/1.1675021" @default.
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