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- W2036724452 abstract "The physical theory necessary for interpreting the vibrational spectra of spin-degenerate molecules is developed in this paper. Particular attention is paid to those molecules whose behaviour is expected to be markedly different from that of both orbitally non-degenerate molecules and those with purely spatial degeneracy. These include certain Kramers degenerate molecules, whose Raman spectra are expected to contain reverse-polarized contributions, and also tetrahedral and octahedral molecules in fourfold degenerate states. The case of a fourfold degenerate octahedral molecule is investigated in the limits of strong vibronic coupling by one of the Jahn—Teller active vibrations (e g and t 2g ). It turns out that the forbidden t 2u vibration may be infra-red active, that the Raman spectrum may contain reverse-polarized contributions and that both infra-red and Raman spectra may contain strong progressions of bands involving multiple excitations of the vibronically active vibration." @default.
- W2036724452 created "2016-06-24" @default.
- W2036724452 date "1962-10-25" @default.
- W2036724452 modified "2023-09-26" @default.
- W2036724452 title "Studies of the Jahn - Teller effect IV. The vibrational spectra of spin-degenerate molecules" @default.
- W2036724452 doi "https://doi.org/10.1098/rsta.1962.0009" @default.
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