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• W2036736149 abstract "The 193 nm photolysis of acetylene has been used as a source of C2(B'1Σ+g) radicals, which are subsequently detected by laser-induced fluorescence technique. The pressure-dependent collisional lifetimes of this radical are experimentally determined by delaying the probe laser with respect to the photolysis laser, thus allowing extraction of the pseudo-first-order rate constants. Stern—Volmer plots of these rate constants versus pressure yield the natural radiative lifetimes of the state. Three different rotational levels of the C2(B'1Σ+g) state were studied. The natural radiative lifetimes were 11.6±1.4 μs and 10.4±1.9 μs for the ν'=0, J'=8 and J'=14 levels, respectively, and 8.3±1.9 μs for the ν'=1, J'=8 level. These values are in reasonable agreement with the recent theoretical calculations. In addition, the second-order rate constants for the excited state quenching by Ar have also been calculated from the data." @default.
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• W2036736149 date "1994-01-01" @default.
• W2036736149 modified "2023-09-24" @default.
• W2036736149 title "LIF measurements of radiative lifetimes of the C2(B'1Σ+g) state" @default.
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• W2036736149 doi "https://doi.org/10.1016/0009-2614(93)e1374-p" @default.
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