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- W2036736518 abstract "A theory of vibration→ rotation energy transfer, which takes specific account of near resonances between quantized vibrator and rotor energy levels, is derived. This theory is in good agreement with experimental data on the deactivation of BCl3(ν4=1 Δ E=243 cm−1) by HCl and DCl, and in fair agreement with data for BCl3 with H2, HD, and D2. Theories that treat the rotor classically do not adequately predict these transition probabilities. The effect of using a first Born approximation is compared to a two‐level close‐coupled calculation, and the effect of a modified‐wave‐number approximation is examined; neither of these approximations materially affect the results. The PHCl/PDCl ratio is predicted to decrease from large values at low temperatures to nearly unity at higher temperatures." @default.
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- W2036736518 date "1973-04-15" @default.
- W2036736518 modified "2023-10-18" @default.
- W2036736518 title "Near‐resonant vibration↔ rotation energy transfer" @default.
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