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- W2037127555 startingPage "A1552" @default.
- W2037127555 abstract "The diffusion of silver-110 into lead has been investigated using radioactive-tracer techniques in a temperature range within 200ifmmode^circelsetextdegreefi{}C of the melting point of lead for six pressures between 0 and 40 kbar. The activation energy was found to increase from 15.2 to 21.9ifmmodepmelsetextpmfi{}0.3 kcal/mole as the pressure increased from atmospheric to 39.2 kbar. The activation volume for pressures below 11.9 kbar ranged from 0.54ifmmodepmelsetextpmfi{}0.06 to 0.48ifmmodepmelsetextpmfi{}0.05 atomic volumes as the temperature decreased from 769 to 556ifmmode^circelsetextdegreefi{}K. Above 11.9 kbar the activation volume was nearly constant at 0.38ifmmodepmelsetextpmfi{}0.03 atomic volumes over the same temperature interval. As a result of the large decrease in the activation volume that occurs between 0 and 11.9 kbar it is suggested that the diffusion process for silver into lead changes from a composite of interstitial plus vacancy to an interstitial mechanism. Therefore the activation volume of 0.38ifmmodepmelsetextpmfi{}0.03 atomic volumes as measured for pressures above 11.9 kbar represents the activation volume of motion $ensuremath{Delta}{V}_{m}$ characterizing the interstitial mechanism. Within the accuracy of the experimental data for $mathrm{ln}D$ versus $frac{{T}_{m}}{T}$ the results suggest that $frac{ensuremath{Delta}H(P)}{{T}_{m}(P)}$ is independent of pressure to 40 kbar." @default.
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- W2037127555 date "1965-08-30" @default.
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- W2037127555 title "Effect of Pressure on the Intermetallic Diffusion of Silver in Lead" @default.
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- W2037127555 doi "https://doi.org/10.1103/physrev.139.a1552" @default.
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