FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2037141206> ?p ?o ?g. }

• W2037141206 endingPage "602" @default.
• W2037141206 startingPage "597" @default.
• W2037141206 abstract "Accurate measurement of the 240Pu/239Pu ratio in environmental samples is of importance as it may provide evidence for the definitive identification of a particular source-term. Usually, the measurement is performed by mass spectrometry, unless the activities involved are relatively high. In such cases, as the published literature shows, it is feasible to determine this ratio using high resolution alpha spectrometry and appropriate algorithms to deconvolute the partially resolved 239,240Pu multiplet. In this paper, a simple technique, based on commercially-available software developed for gamma spectra analysis (MicroSAMPO®), is described by which this complex multiplet can be resolved at the much lower activities typical of many environmental samples. In our approach, it is not necessary to make any alterations to the normal alpha spectrometric set-up (including energy dispersion), other than to improve collimation. The instrumental function is defined for each spectrum by fitting a modified gaussian with exponential tails to the comparatively well-resolved 242Pu “doublet” (used as tracer) and, if present, the 238Pu “doublet”. The fitted peaks are used to create an energy calibration file with which, using published energy data, the positions (in channels) of the component peaks of the multiplet are predicted. These positions are not altered subsequently when MicroSAMPO's interactive multiplet analysis facility is used to quantify the relative spectral intensities of the components. Before calculating the 240Pu/239Pu ratio, it is advisable to correct for coincidence summing of alpha particles and conversion electrons. The technique has been applied to the determination of the 240Pu/239Pu ratio in a set of environmental samples, most of which were supplied by IAEA-MEL under their laboratory intercomparison programme. Subsequently, replicate samples were analysed independently using thermal ionisation mass spectrometry. The agreement between the two sets of data was most satisfactory. Further validation of this deconvolution technique was provided by the good agreement between the measured alpha-emission probabilities for the component peaks in the 239, 240Pu multiplet and published values." @default.
• W2037141206 created "2016-06-24" @default.
• W2037141206 creator A5046427414 @default.
• W2037141206 creator A5048244312 @default.
• W2037141206 creator A5058027403 @default.
• W2037141206 creator A5072363661 @default.
• W2037141206 creator A5073463096 @default.
• W2037141206 creator A5091190579 @default.
• W2037141206 date "1996-02-01" @default.
• W2037141206 modified "2023-10-01" @default.
• W2037141206 title "Determination of the 240Pu/239Pu atom ratio in low activity environmental samples by alpha spectrometry and spectral deconvolution" @default.
• W2037141206 cites W1549562804 @default.
• W2037141206 cites W1982952104 @default.
• W2037141206 cites W1994786326 @default.
• W2037141206 cites W2025578638 @default.
• W2037141206 cites W2032578455 @default.
• W2037141206 cites W2042020289 @default.
• W2037141206 cites W2043964842 @default.
• W2037141206 cites W2051766640 @default.
• W2037141206 cites W2052302722 @default.
• W2037141206 cites W2053863922 @default.
• W2037141206 cites W2063383669 @default.
• W2037141206 cites W2076944860 @default.
• W2037141206 cites W2078973837 @default.
• W2037141206 cites W2079226641 @default.
• W2037141206 cites W2085299637 @default.
• W2037141206 cites W2090930824 @default.
• W2037141206 cites W3093240389 @default.
• W2037141206 cites W4251500648 @default.
• W2037141206 doi "https://doi.org/10.1016/s0168-9002(96)80059-3" @default.
• W2037141206 hasPublicationYear "1996" @default.
• W2037141206 type Work @default.
• W2037141206 sameAs 2037141206 @default.
• W2037141206 citedByCount "28" @default.
• W2037141206 countsByYear W20371412062012 @default.
• W2037141206 countsByYear W20371412062013 @default.
• W2037141206 countsByYear W20371412062014 @default.
• W2037141206 countsByYear W20371412062020 @default.
• W2037141206 countsByYear W20371412062021 @default.
• W2037141206 countsByYear W20371412062022 @default.
• W2037141206 crossrefType "journal-article" @default.
• W2037141206 hasAuthorship W2037141206A5046427414 @default.
• W2037141206 hasAuthorship W2037141206A5048244312 @default.
• W2037141206 hasAuthorship W2037141206A5058027403 @default.
• W2037141206 hasAuthorship W2037141206A5072363661 @default.
• W2037141206 hasAuthorship W2037141206A5073463096 @default.
• W2037141206 hasAuthorship W2037141206A5091190579 @default.
• W2037141206 hasConcept C113196181 @default.
• W2037141206 hasConcept C120665830 @default.
• W2037141206 hasConcept C121332964 @default.
• W2037141206 hasConcept C1276947 @default.
• W2037141206 hasConcept C133871045 @default.
• W2037141206 hasConcept C134306372 @default.
• W2037141206 hasConcept C138268822 @default.
• W2037141206 hasConcept C151376022 @default.
• W2037141206 hasConcept C154945302 @default.
• W2037141206 hasConcept C162356407 @default.
• W2037141206 hasConcept C165838908 @default.
• W2037141206 hasConcept C174576160 @default.
• W2037141206 hasConcept C184779094 @default.
• W2037141206 hasConcept C185592680 @default.
• W2037141206 hasConcept C30475298 @default.
• W2037141206 hasConcept C33923547 @default.
• W2037141206 hasConcept C41008148 @default.
• W2037141206 hasConcept C43617362 @default.
• W2037141206 hasConcept C4839761 @default.
• W2037141206 hasConcept C62520636 @default.
• W2037141206 hasConceptScore W2037141206C113196181 @default.
• W2037141206 hasConceptScore W2037141206C120665830 @default.
• W2037141206 hasConceptScore W2037141206C121332964 @default.
• W2037141206 hasConceptScore W2037141206C1276947 @default.
• W2037141206 hasConceptScore W2037141206C133871045 @default.
• W2037141206 hasConceptScore W2037141206C134306372 @default.
• W2037141206 hasConceptScore W2037141206C138268822 @default.
• W2037141206 hasConceptScore W2037141206C151376022 @default.
• W2037141206 hasConceptScore W2037141206C154945302 @default.
• W2037141206 hasConceptScore W2037141206C162356407 @default.
• W2037141206 hasConceptScore W2037141206C165838908 @default.
• W2037141206 hasConceptScore W2037141206C174576160 @default.
• W2037141206 hasConceptScore W2037141206C184779094 @default.
• W2037141206 hasConceptScore W2037141206C185592680 @default.
• W2037141206 hasConceptScore W2037141206C30475298 @default.
• W2037141206 hasConceptScore W2037141206C33923547 @default.
• W2037141206 hasConceptScore W2037141206C41008148 @default.
• W2037141206 hasConceptScore W2037141206C43617362 @default.
• W2037141206 hasConceptScore W2037141206C4839761 @default.
• W2037141206 hasConceptScore W2037141206C62520636 @default.
• W2037141206 hasIssue "2-3" @default.
• W2037141206 hasLocation W20371412061 @default.
• W2037141206 hasOpenAccess W2037141206 @default.
• W2037141206 hasPrimaryLocation W20371412061 @default.
• W2037141206 hasRelatedWork W1992788792 @default.
• W2037141206 hasRelatedWork W1999916039 @default.
• W2037141206 hasRelatedWork W2019288765 @default.
• W2037141206 hasRelatedWork W2025121688 @default.
• W2037141206 hasRelatedWork W2026642978 @default.
• W2037141206 hasRelatedWork W2028531314 @default.
• W2037141206 hasRelatedWork W2080147620 @default.

• next