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• W2037165788 endingPage "1183" @default.
• W2037165788 startingPage "1175" @default.
• W2037165788 abstract "Six new mixed-ligand coordination polymers, namely, [Zn(1,3-bdc)(3-bpdb)]n (1), {[Zn(1,3-bdc)(4-bpdb)]·2H2O}n (2), [Co(1,4-bdc)(3-bpdb)(H2O)2]n (3), [Ni(1,4-bdc)(3-bpdb)(H2O)]n (4), {[Co5(1,4-ndc)4(3-bpdb)(μ3-OH)2(H2O)2(DMF)2]·2H2O·CH3OH}n (5), and {[Zn2(1,4-ndc)2(3-bpdb)]·H2O}n (6), where 3-bpdb = 1,4-bis(3-pyridyl)-2,3-diaza-1,3-butadiene, 4-bpdb = 1,4-bis(4-pyridyl)-2,3-diaza-1,3-butadiene, 1,3-H2bdc = 1,3-benzenedicarboxylic acid, 1,4-H2bdc = 1,4-benzenedicarboxylic acid, and 1,4-H2ndc = 1,4-naphthalenedicarboxylic acid, were synthesized under solvothermal conditions. Single crystal X-ray diffraction analysis revealed that the structures of complexes 1 and 2 were isomorphic and exhibited two-dimensional (2D) double-layered sql nets. Complex 3 had an interesting 2D → three-dimensional (3D) inclined polycatenation net based on 44-sql subunits. Complex 4 featured an uncommon 3D 2-fold cds network, while complex 5 possessed a rare uninodal self-penetrating 10-connected pentacobalt-cluster-based ile-(36.434.53.62) framework. Complex 6 displayed a 2-fold interpenetrated 3D six-connected pcu topology. These different intriguing architectures indicated that the coordination behaviors of metal ions and the coordination modes, the position isomers of carboxylate, and different steric hindrances of aromatics played important roles in the construction of CPs; moreover, bpdb ligands with conformational freedom may affect the formation of the final architectures. The photoluminescence properties of 1, 2, and 6 in the solid state and the magnetic properties of 5 were studied. Moreover, thermal analysis, powder X-ray diffraction, infrared spectroscopy, and elemental analysis were also performed." @default.
• W2037165788 created "2016-06-24" @default.
• W2037165788 creator A5005305428 @default.
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• W2037165788 creator A5025636973 @default.
• W2037165788 creator A5029695887 @default.
• W2037165788 creator A5070358168 @default.
• W2037165788 creator A5078865346 @default.
• W2037165788 date "2014-02-14" @default.
• W2037165788 modified "2023-09-25" @default.
• W2037165788 title "Intriguing Architectures Generated from 1,4-Bis(3- or 4-pyridyl)-2,3-diaza-1,3-butadiene with Aromatic Dicarboxylates: Syntheses, Crystal Structures, and Properties" @default.
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