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• W2037516516 abstract "Selective cleaving of both O–H and O–D bonds in HOD is achieved using reasonably simple UV pulses to excite the HOD molecule in its ground vibrational state to the repulsive first excited Ã(B11) surface. Detailed theoretical analysis of population transfer and flux in theH+O–D∕H–O+D channels reveals an important preparatory role for the cross-talk between the participating levels and a possible role for the beat structure of the population transfer oscillations in facilitating selective dissociation. Excitation using a 50fs single color 67169cm−1 laserpulse achieves a branching ratio H+O–D∕H–O+D=5.64 with 82% flux in theH+O–D channel and 15% in the H–O+D channel. A two color 50fs laser pulse with frequencies of 54 920 and 52303cm−1 provides a branching ratio of H–O+D∕H+O–D=2.83 and 52% flux in the H–O+D channel and 18% in the H+O–D channel." @default.
• W2037516516 created "2016-06-24" @default.
• W2037516516 creator A5001424167 @default.
• W2037516516 creator A5010626819 @default.
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• W2037516516 date "2007-07-12" @default.
• W2037516516 modified "2023-09-27" @default.
• W2037516516 title "Selective photodissociation of O–H and O–D bonds from ground vibrational state of HOD using simple UV pulses" @default.
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• W2037516516 doi "https://doi.org/10.1063/1.2751185" @default.
• W2037516516 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17640126" @default.
• W2037516516 hasPublicationYear "2007" @default.
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