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- W2037744553 abstract "Elastic models imply that the energy expended for a flow event in ultra-viscous matter coincides with the elastic work required for deforming and re-arranging the environment of the moving entity. This is quite promising for explaining the strong non-Arrhenius behavior of dynamic quantities of fragile super-cooled liquids. We argue that the activation volume obtained from dielectric relaxation and light-scattering experiments for super-cooled liquids should scale with the Gibbs free energy of activation, with a proportionality constant determined by the isothermal bulk modulus and its pressure derivative, as described by an earlier thermodynamic elastic model. For certain super-cooled liquids the bulk compression transpiring in the local environment, as governed by the isothermal bulk modulus, play a significant role in the reorientational dynamics, with far-field density fluctuations and volume changes avoided by shear deformation." @default.
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- W2037744553 date "2011-12-28" @default.
- W2037744553 modified "2023-09-25" @default.
- W2037744553 title "The role of the isothermal bulk modulus in the molecular dynamics of super-cooled liquids" @default.
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- W2037744553 doi "https://doi.org/10.1063/1.3666008" @default.
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