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- W2037800346 abstract "Resonant two-photon ionization spectroscopy has been used to investigate the optical spectra of jet-cooled MoO. By coupling the technique to a time-of-flight mass spectrometer, spectra of 92Mo16O, 94Mo16O, 95Mo16O, 96Mo16O, 97Mo16O, 98Mo16O, and 100Mo16O have been separately recorded. The observed spectra establish the ground state of MoO as 5Πr, deriving from the 2δ212σ16π1 molecular configuration. Transitions from this ground state to the excited 1δ112σ16π2, A′5Δr; 2δ26π113σ1, B5Πr; and 2δ112σ16π113π1, B′5Πr states have been located, rotationally resolved, and analyzed. Numerous other weak transitions have been observed in the visible, many of which must be due to S = 1 ← X5Πr intercombinations. Several strong transitions are observed in the near infrared where the 2δ212σ113σ1, 5Σ− ← X5Π and 2δ26π2, A5Σ+ ← X5Π band systems are expected. The general electronic structure of MoO is shown to be quite analogous to that of its congener, CrO, and the pattern of molecular orbital energies is also quite comparable to that found for NbO." @default.
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- W2037800346 date "1991-04-01" @default.
- W2037800346 modified "2023-10-14" @default.
- W2037800346 title "Optical spectroscopy of jet-cooled MoO" @default.
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- W2037800346 doi "https://doi.org/10.1016/0022-2852(91)90005-u" @default.
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