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- W2037861791 abstract "Abstract Kinetic and equilibrium properties of water adsorption by plutonium dioxide are derived from gravimetric measurements in moist air at room temperature. In combination with mass–time data extracted from literature sources, the results provide a comprehensive picture of the adsorption process and its humidity dependence at 25 °C. Water is accommodated by a sequence of distinct steps involving five types of adsorbate–oxide interaction and accumulating ten molecular layers of water (approximately 2.1 mg H2O/m2 PuO2 surface) at 100% relative humidity. The humidity-dependent first step and the second step involve half molecular layers of water and are attributed to dissociative chemisorption of water as OH. Like the second step, all subsequent processes are first order, but each involves a single molecular layer of H2O. Kinetic and equilibrium results are applied in defining conditions for limiting the re-adsorption of water during handling operations and their relevance to the complex chemistry of the plutonium–oxygen system is outlined." @default.
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- W2037861791 date "1997-05-01" @default.
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- W2037861791 title "Adsorption of water on plutonium dioxide" @default.
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- W2037861791 doi "https://doi.org/10.1016/s0925-8388(96)02627-8" @default.
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