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• W2037995989 startingPage "A1599" @default.
• W2037995989 abstract "Nonlinear optical polarization quadratic in the optical electric fields is shown to occur in optically active liquids and to lead to sum- and difference-frequency generation; second-harmonic generation is forbidden. The nonlinearity is described by components of the second-order polarizability tensor ${ensuremath{chi}}_{mathrm{ijk}}$ antisymmetric in $j$ and $k$; the form of the antisymmetric part of ${ensuremath{chi}}_{mathrm{ijk}}$ is given for all the crystal classes and textures and for isotropic media. The magnitude of nonlinear polarizability of liquids is estimated from second-order perturbation theory and calculated to be readily detectable in many optically active liquids. The mechanism of the nonlinearity is illustrated by a simple single-electron molecular model." @default.
• W2037995989 created "2016-06-24" @default.
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• W2037995989 date "1965-06-14" @default.
• W2037995989 modified "2023-09-26" @default.
• W2037995989 title "Nonlinear Optical Properties of Liquids" @default.
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• W2037995989 doi "https://doi.org/10.1103/physrev.138.a1599" @default.
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