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- W2038036353 abstract "We investigate the quantum optical properties of an excited single photon emitter (quantum dot) near thesurface of a finite-size metal nanoparticle using a photon Green function technique that rigorously quantizes theelectromagnetic fields. We obtain Purcell factors of up to 5×10 4 due to higher order plasmon modes for both a7-nm and 20-nm radius metal nanoparticle, and show the failure of employing a dipole approximation in regimeswhere useful quantum optical interactions occur. We also calculate enormous photonic Lamb shifts of up to40 meV giving a normalized frequency shift up to |Δω| max /ω d = 1.28×10 -2 . Considering a small quantum-dot,positioned 2-nm from the metal nanoparticle surface, we demonstrate that the strong coupling regime shouldbe observable in the far-field spontaneous emission spectrum, even at room temperature and despite the non-propagatingnature of the higher order modes. The vacuum Rabi doublet becomes a rich spectral quartet withtwo of the four peaks anticrossing, and surviving in spite of significant non-radiative decays. We also discuss therole of optical quenching and highlight the importance of accounting for photon transport from the dot to thedetector. Our formalism is quite general and can easily be extended to include interactions between multiplequantum dots and multiple metal nanoparticles." @default.
- W2038036353 created "2016-06-24" @default.
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- W2038036353 date "2012-04-30" @default.
- W2038036353 modified "2023-09-25" @default.
- W2038036353 title "Nonpeturbative cavity-QED between a single quantum dot and a metal nanoparticle" @default.
- W2038036353 doi "https://doi.org/10.1117/12.922557" @default.
- W2038036353 hasPublicationYear "2012" @default.
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