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- W2038231736 abstract "Exposure of CuSSZ13 to CO2 at temperatures below 300 °C can deactivate its low-temperature deNOx activity during NH3/SCR, with the severity of deactivation being dependent on reaction temperature. The adsorption of NO on Cu2+ ion is inhibited by CO2 due to its competitive adsorption, while NH3 adsorption on acidic sites of CuSSZ13 is largely unaffected by CO2, as evidenced by NO- and NH3-TPD in the presence of CO2. Under O2-rich conditions, CO2 forms unidentate carbonates on Cu2+ sites suppressing the formation of nitrates, a key reaction intermediate essential for NOx reduction during the NH3/SCR reaction, as revealed in an in situ FTIR study." @default.
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- W2038231736 date "2014-03-11" @default.
- W2038231736 modified "2023-10-07" @default.
- W2038231736 title "Effect of CO2on the DeNOxActivity of a Small Pore Zeolite Copper Catalyst for NH3/SCR" @default.
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- W2038231736 doi "https://doi.org/10.1002/cctc.201400093" @default.
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