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• W2038406056 endingPage "2687" @default.
• W2038406056 startingPage "2680" @default.
• W2038406056 abstract "Emission of the CO Fourth Positive Bands (A 1π–X 1Σ+) is observed in the reactions of atomic N/O mixtures with C2F4, C2H4, C2H2, and C2N2 at about 300°K and pressures of 1–4 Torr. The N/O/C2F4 system, which has been investigated most extensively, produces CO A 1π–X 1Σ+ emission which, like the NO+ chemi-ion formation rate, follows [N]3[O] kinetics. The level of excitation extends to at least 10.3 eV above CO(X 1Σ+, υ = 0). It is shown that the formation of CO(A 1π) can be attributed to enhanced formation of excited N2 and NO molecules in atom-recombination reactions induced by a reaction intermediate (probably CN), followed by pooling of the energy of an N2* and an NO* molecule and energy transfer to the reaction product CO(X 1Σ+). The transfer reaction can take place before or after the pooling reaction. Formation of CO(A 1π) in the N/O/C2H4 system exhibits the same kinetic dependence on N and O atoms. For the N/O/C2H2 system, the observations indicate CO(A 1π) formation both via the above energy-pooling mechanism and via the mechanism operative in the O/C2H2 reaction [O+C2O→CO(A 1π)+CO(X 1Σ+)]. In the N/O/C reactions, the higher vibrational levels of CO(A 1π) are relatively more populated than in the O/C2H2 reaction." @default.
• W2038406056 created "2016-06-24" @default.
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• W2038406056 date "1970-10-01" @default.
• W2038406056 modified "2023-09-24" @default.
• W2038406056 title "Chemiluminescent Emission of CO Fourth Positive Bands in Nitrogen Atom/Oxygen Atom/Reactive Carbon Compound Systems. Relation to Chemi-ionization" @default.
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• W2038406056 doi "https://doi.org/10.1063/1.1674391" @default.
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