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• W2038512634 abstract "A recent theory of time-resolved X-ray diffraction is used to show how atomic motions in chemical reactions can be monitored. Only quasi-static reactions which evolve slowly as compared to the time scale of laser excitation are considered. The general expression for the X-ray signal is expressed in terms of temporally varying pair distribution functions, and a procedure is described to extract them from time resolved X-ray experiments. The density changes induced by laser heating are also included into the theory, and their signature is discussed. New experimental results concerning the I2/CCl4 solution are reported. The recombination of the laser-dissociated iodine is monitored at pico- and nanosecond time scales. The CCl4 molecules take part of the reaction; the solvent thus appears as a reaction partner rather then an inert medium hosting it." @default.
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• W2038512634 date "2004-10-01" @default.
• W2038512634 modified "2023-09-26" @default.
• W2038512634 title "X-ray “filming” of atomic motions in chemical reactions" @default.
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• W2038512634 doi "https://doi.org/10.1016/j.chemphys.2004.06.065" @default.
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