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W2038777291 abstract "The absorption spectrum of the linear→bent 1Σ+g→1B2 (1Σ+u) transition of jet-cooled CS2 is reported in the 47 750–53 200 cm−1 region. Adjustment of diluent gas composition enables the preparation of rotationally cold (<10 K)/vibrationally hot (≊300 K) and rotationally cold/vibrationally cold samples. The collapse of rotational envelopes on cooling facilitates the accurate determinations of frequencies and relative absorption intensities of transitions both from the zero point level and from excited vibrational levels of the ground electronic state. At 49 000–51 000 cm−1, in the region of the Franck–Condon maximum, a simple vibronic pattern emerges involving two upper state vibrational modes containing both stretching and bending contributions. In this region of the spectrum, the upper state rotational structure diverges from that of a nearly symmetric top and approaches that of the linear or quasilinear molecule. At higher energies, the vibronic structure grows in complexity, suggesting increased anharmonic mixing of these nearly degenerate modes." @default.
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W2038777291 date "1983-12-01" @default.
W2038777291 modified "2023-09-23" @default.
W2038777291 title "The direct ultraviolet absorption spectrum of the 1Σ+g→ 1B2(1Σ+u) transition of jet-cooled CS2" @default.
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W2038777291 doi "https://doi.org/10.1063/1.445710" @default.
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