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- W2038818097 abstract "Abstract Solvatochromic behavior of acetone in supercritical CO 2 was investigated over a wide range of pressures from 75 to 240 bar and at 318.15 K using UV‐Vis spectroscopy. Local density of CO 2 about the solute was estimated from the solvatochromic shift of acetone based on the McRae‐Bayliss dielectric continuum model. The most remarkable aggregation of CO 2 about the solute occurs at the reduced density of 0.5 ∼ 0.6. A simple clustering model was presented to estimate the excess solvent number about each solute molecule to the bulk region. In the near‐critical region, the excess number of CO 2 is larger than the cluster size at infinite dilution defined by Debenedetti, which may be attributed to the formation of solute‐solute clusters." @default.
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- W2038818097 date "1998-04-01" @default.
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- W2038818097 title "UV-Vis spectroscopic study of molecular clustering in supercritical CO2-acetone mixtures" @default.
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- W2038818097 doi "https://doi.org/10.1002/bbpc.19981020414" @default.
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