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- W2038863011 abstract "Depending on the iron(ii) concentration, the mixed crystals of {[Zn1-xFex(bbtr)3](BF4)2}∞, bbtr = 1,4-di(1,2,3-triazol-1-yl)butane, 0.01 ≤ x ≤ 1, show macroscopic light-induced bistability between the high-spin and the low-spin state. In the highly diluted system with x = 0.01 and up to x = 0.31, the photoinduced low-spin state always relaxes back to the high-spin state independent of the initial light-induced low-spin fraction. In the highly concentrated mixed crystals with x = 0.67, 0.87 and 1, the strong cooperative effects coupled to a crystallographic phase transition result in light-induced bistability with decreasing critical light-induced low-spin fraction and increasing hysteresis width for increasing iron(ii) concentrations. The lower limit for the light-induced bistability was estimated to be x ≈ 0.5." @default.
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- W2038863011 date "2014-01-01" @default.
- W2038863011 modified "2023-09-29" @default.
- W2038863011 title "Light-induced spin-state switching in the mixed crystal series of the 2D coordination network {[Zn<sub>1−x</sub>Fe<sub>x</sub>(bbtr)<sub>3</sub>](BF<sub>4</sub>)<sub>2</sub>}<sub>∞</sub>: optical spectroscopy and cooperative effects" @default.
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- W2038863011 doi "https://doi.org/10.1039/c4dt01728e" @default.
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