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- W2039051323 abstract "The effectiveness of energy conversion and carbon dioxide sequestration in Integrated GasificationCombined Cycle (IGCC) is highly dependent on the syngas composition and its further processing. Watergas shift membrane reactor (WGSMR) enables a promising way of syngas-to-hydrogen conversion withfavourable carbon dioxide sequestration capabilities. This paper deals with a numerical approach tothe modelling of a water gas shift reaction (WGSR) in a membrane reactor which promotes a reactionprocess by selectively removing hydrogen from the reaction zone through the membrane, making thereaction equilibrium shifting to the product side. Modelling of the WGSR kinetics was based on Bradfordmechanism which was used to develop a code within Mathematica programming language to simulatethe chemical reactions. The results were implemented as initial and boundary conditions for the tubularWGSMR model designed with Aspen Plus software to analyze the broader system behaviour. On the basisof selected boundary conditions the designed base case model predicts that 89.1% CO conversion can beachieved. Calculations show that more than 70% of carbon monoxide conversion into hydrogen appearsalong the first 40% of reactor length scale. For isothermal conditions more than two thirds of the heatreleased by WGSR should be extracted from the first 20% of the reactor length. Sensitivity analysis of theWGSMR was also performed by changing the membrane’s permeance and surface area." @default.
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- W2039051323 date "2011-12-15" @default.
- W2039051323 modified "2023-10-14" @default.
- W2039051323 title "Simulation of Water-Gas Shift Membrane Reactor for Integrated Gasification Combined Cycle Plant with CO2 Capture" @default.
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- W2039051323 doi "https://doi.org/10.5545/sv-jme.2011.100" @default.
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