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- W2039068169 abstract "Abstract The hydrogen absorption/desorption kinetics and P–C isotherm of Mg 70 (Ni 0.75 La 0.25 ) 30 alloy, both the as-melt and rapid solidification were carried out on a sievert-type apparatus. The experimental data of initial hydrogen absorption and desorption kinetics at 573 K are in good agreement with Avrami–Erofeev equation, which indicated a three-dimensional interface reaction process of nucleation and growth for the initial hydrogenation kinetics and ‘‘geometrical contraction model’’ for dehydrogenation kinetics. However, the third absorption process seems to have a different hydriding mechanism as chemical reaction. P–C isotherm curves show that the as-melt alloy has two distinct hydrogen absorption plateaus, while the rapid solidification alloy has only one, which attribute to the absent of LaMg 3 phase by rapid solidification. It can be confirmed by DSC analysis that the as-melt alloy has two endothermic peaks, compared to one for the rapid solidification alloy. The dehydrogenation activation energies of Mg 70 (Ni 0.75 La 0.25 ) 30 alloy were calculated by Kissinger method, showing the values of 128.60 ± 13.79 and 112.89 ± 9.94 kJ/mol for the as-melt sample and 61.09 ± 6.28 kJ/mol for rapid solidification alloy respectively." @default.
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- W2039068169 date "2012-09-01" @default.
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- W2039068169 title "Effect of rapid solidification on phase structure and hydrogen storage properties of Mg70(Ni0.75La0.25)30 alloy" @default.
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- W2039068169 doi "https://doi.org/10.1016/j.ijhydene.2012.03.133" @default.
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