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- W2039392718 abstract "It is shown that, under an intense high-frequency laser field, electronic distributions in molecules exhibit a dichotomy effect just as previously found in atoms. The generalization of the formal demonstration of the dichotomy effect as given in M. Gavrila and J. Shertzer, Phys. Rev. A 41, 477 (1990) to many-electron, polyatomic molecules is considered and the validity of the α0−2/3 scaling law of the Floquet eigenvalues, with respect to the field intensity parameter α0 of the HFFT, is discussed. To test the molecular dichotomy effect, numerical calculations are performed using a quantum chemical package (Gaussian 94), modified appropriately to incorporate the cycle-averaged displacements of the nuclear–electron Coulomb potential as found in the HFFT hamiltonian. Results of calculations on the two-electron H2 molecule are presented with an emphasis placed on the character of the total and orbital charge distributions and on trends to be observed in the electronic correlation at high intensities." @default.
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- W2039392718 date "2000-01-15" @default.
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- W2039392718 title "Molecular dichotomy within an intense high-frequency laser field" @default.
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