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- W2039423056 abstract "A technique has been established to determine the first hyperpolarizability value β of fluorescent molecules based on femtosecond hyper-Rayleigh scattering (HRS). The intrinsic high harmonic content of the femtosecond pulse train is used as a high frequency amplitude modulation source. Due to the nonzero fluorescence lifetime, a high amplitude modulation frequency will result in an amplitude demodulated and phase shifted fluorescence signal. At very high modulation frequencies, the fluorescence signal becomes completely demodulated and only the inherent HRS signal will remain. A comparative study was made between the dispersion free β0-value of a nonfluorescent ionic hemicyanine dye (DASPC22+) and the dispersion free β0-value of the fluorescent inclusion complex of the dye incorporated in an amylose matrix. The fluorescence-free β0-value for the complex appeared to be twice [(200 ± 5) × 10−30 esu] the β0-value of the dye itself [(100 ± 10) × 10−30 esu]." @default.
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- W2039423056 date "1999-06-01" @default.
- W2039423056 modified "2023-09-25" @default.
- W2039423056 title "High-frequency demodulation of multi-photon fluorescence in hyper-Rayleigh scattering" @default.
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- W2039423056 doi "https://doi.org/10.1016/s0925-3467(99)00060-9" @default.
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