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• W2039432352 abstract "Several donor-sigma acceptor (D-sigma-A) molecules with thioalkyl side chains have been prepared by ruthenium-activated nucleophilic aromatic substition (S(N)Ar) reactions. Selective substitution of chloride from cyclopentadienyl(1,4-dichlorobenzene)ruthenium by using piperazine derivatives as nucleophiles is addressed. This selectivity, in combination with further manipulation of the complexes, allows the preparation of unsymmetrically functionalized tetraalkyl-p-phenylenediamine (TAPD) units which are difficult to synthesize by traditional organic S(N)Ar conditions. Phenanthroline-assisted decomplexation of the product arene-RuCp systems under UV irradiation is described." @default.
• W2039432352 created "2016-06-24" @default.
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• W2039432352 date "2000-05-10" @default.
• W2039432352 modified "2023-10-06" @default.
• W2039432352 title "Preparation of Donor-σ-Acceptor Molecules Using Arene−Ruthenium Chemistry" @default.
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• W2039432352 doi "https://doi.org/10.1021/jo000018s" @default.
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