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• W2039457293 abstract "A high yield of the tetraphosphaladderene, anti-tetraphosphatricyclo[4.2.0.02,5]octa-3,7-diene, is obtained from reaction of the zirconocene 1,3-diphosphabicyclo[1.1.0]butane with Ph2SbCl3 in THF or CH2Cl2. Exploration of the reaction pathway using density functional theory suggests that an envelope-type adduct of Ph2SbCl and 1,3-diphosphabicyclo[1.1.0]butane plays a pivotal role in the reaction. The zwitterionic character of this intermediate species allows it to act simultaneously as both an ene and an eneophile, and a symmetry-allowed bimolecular reaction leads to the tetraphosphaladderene species via a spirocyclic intermediate." @default.
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• W2039457293 date "2008-01-01" @default.
• W2039457293 modified "2023-09-25" @default.
• W2039457293 title "Promotion of phosphaalkyne cyclooligomerisation by a Sb(v) to Sb(iii) redox process" @default.
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• W2039457293 doi "https://doi.org/10.1039/b804401e" @default.
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