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- W2039482609 abstract "The energy transfer between a pair of excited Na(3p) atoms leading to Na(3s)+Na(5s) and Na(3s)+Na(4d) final states is studied in a semiclassical coupled-state theory. Classical trajectories are evaluated from the average adiabatic potentials of previously calculated excited molecular states of ${mathrm{Na}}_{2}$. With this specification of average nuclear R(t) for atoms approaching in a given magnetic quantum number (${m}_{a}$,${m}_{b}$) substate, we solve the coupled equations for the time-dependent Schrodinger equation in the 21-state diabatic basis set (including 3p, 3s, 5s, and 4d) of atom pairs. The coupling terms arise from the dipole-dipole interaction. Excellent agreement is obtained with the data of the two most recent measurements of the 3s+4d and 3s+5s energy-transfer cross sections at Tensuremath{sim}500--600 K. Extension to low temperature shows a rising 3s+5s cross section as a result of a net attractive adiabatic potential in the (${m}_{a}$,${m}_{b}$)=(1,0) incident channel, as also occurs for associative ionization." @default.
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- W2039482609 date "1989-09-01" @default.
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- W2039482609 title "Theory of energy-transfer collisions of excited sodium atoms: 3P+3P→3S+5S or 4D" @default.
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- W2039482609 doi "https://doi.org/10.1103/physreva.40.2301" @default.
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