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- W2039843904 abstract "Liquid crystalline ordering in planar polymer brushes is investigated theoretically by numerical calculations within a self-consistent field approximation. The brushes are formed by macromolecules with mesogenic groups in main chain and immersed in a solvent. Existence of a microphase segregated brush (MSB) regime with a collapsed orientationally ordered intrinsic sublayer and a swollen external sublayer is shown. At small grafting density, the transition from a conventional brush state to the microphase segregated state is a jump-wise first order phase transition for a finite chain length (N). The magnitudes of the jumps in the average characteristics of the brush tend to zero in the limit N → ∞ since this transition occurs only in a vanishingly small part (∝ N−1/2) of the brush. High compressibility of MSB brush is demonstrated. The origin of phase transition in planar brushes is discussed." @default.
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- W2039843904 date "1997-02-01" @default.
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- W2039843904 title "Phase transitions in polymer brushes" @default.
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- W2039843904 doi "https://doi.org/10.1002/masy.19971130114" @default.
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