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- W2039919100 abstract "Abstract Starting from recently observed beating patterns in trans-stilbene we consider the correspondence of classical molecular dynamics and quantum dynamics for the description of the internal vibrational energy redistribution in molecules. The beat frequency of two modes in 2:1 resonance is investigated with respect to quantum effects, sensitivity to anharmonic coupling and indirect coupling via a third oscillator. We find a robust correspondence between classical and quantum beat frequencies but a large sensitivity to the coupling terms in the potential. Refined anharmonic coupling appears to be needed to resolve the very low frequency beating patterns observed in trans-stilbene." @default.
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- W2039919100 date "1996-06-01" @default.
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- W2039919100 title "Beats in internal vibrational energy redistribution in trans-stilbene — A study of the quantum and classical correspondence" @default.
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- W2039919100 doi "https://doi.org/10.1016/0301-0104(96)00034-1" @default.
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