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- W2040229189 abstract "A mechanism of attraction between like-charged macroions due to charge fluctuation has been revisited for macroions of different geometries. For higher charge asymmetry, macroion geometry plays an important role in charge fluctuation, while for comparatively lower charge asymmetry the fluctuation is almost independent of the geometry. At very low temperatures and in a high Coulomb coupling regime, stable ionized states due to auto-ionization are able to exist, which leads to long range Coulomb attraction. Overcharging of a single macroion and its counterion distribution minimizing the total energy has been studied briefly to explain the attraction properties between two like-charged macroions. The investigations have been carried out using a technique based on total energy minimization which has been verified successfully for some special cases with molecular dynamics simulation results previously published. A theoretical model, derived by modifying the Scatchard approach, is proposed to explain the overcharging curves obtained from the simulation. It has been found that the model is equally efficient for both spherical and non-spherical macroion geometries. Wigner crystal theory has also been employed for spherical cases, and excellent agreement has been found between the two theoretical approaches." @default.
- W2040229189 created "2016-06-24" @default.
- W2040229189 creator A5016249677 @default.
- W2040229189 date "2004-04-09" @default.
- W2040229189 modified "2023-09-23" @default.
- W2040229189 title "The attraction between like-charged macroions—the crucial roles of macroion geometry and charge distribution" @default.
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- W2040229189 doi "https://doi.org/10.1088/0953-8984/16/16/015" @default.
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