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• W2040262488 endingPage "6712" @default.
• W2040262488 startingPage "6704" @default.
• W2040262488 abstract "The model mixed surfactant system of sodium perfluorooctanoate and sodium decyl sulfate was carefully reexamined by a combination of nuclear magnetic resonance methods. Over a wide range of sample compositions, detailed 19F and 1H chemical shift data in combination with self-diffusion coefficients for the perfluorooctanoate and decyl sulfate ions are collected. All data are analyzed together in a framework that uses a minimal number of initial assumptions to extract the monomer concentrations of both surfactants and the micellar chemical shifts of 19F and 1H as a function of relative concentration. The main conclusion drawn from this analysis is that there exists neither complete demixing nor complete mixing on molecular or micellar levels. Instead, the experimental data favor a single type of micelles within which fluorinated surfactants are preferentially coordinated by fluorinated ones and hydrogenated surfactants by hydrogenated ones. The data are quantitatively interpreted in the framework of the first approximation of the regular solution theory (also called the quasi-chemical treatment) leading to an energy of mixing of ω = W/kT = 0.98 between the constituting surfactant types. These findings may help to resolve a long controversy about micellar mixing−demixing in this particular mixture and in its relatives." @default.
• W2040262488 created "2016-06-24" @default.
• W2040262488 creator A5001159621 @default.
• W2040262488 creator A5054030272 @default.
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• W2040262488 date "2006-05-01" @default.
• W2040262488 modified "2023-09-30" @default.
• W2040262488 title "Mixed Micelles of Fluorinated and Hydrogenated Surfactants" @default.
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• W2040262488 doi "https://doi.org/10.1021/ja061029r" @default.
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• W2040262488 hasPublicationYear "2006" @default.
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