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- W2040331880 abstract "Abstract The infrared spectrum of natural H3SiF has been recorded in the region of the fundamentals ν3 (875.010 cm−1) and ν6 (729.531 cm−1) with a resolution of 0.0025 and 0.007 cm−1, respectively. A rovibrational analysis has been performed, and 1998 measured nonzero weighted transitions of ν3 (K ≦ 8) and ν6 (K ≦ 18) have been fitted, σ = 3.5 × 10−4 cm−1. The model employed accounts for Δl = Δk = ±2 resonance within ν6 and Coriolis x, y resonance between ν3 and ν6, ζ 3,6 ⋍ −0.341 . Additional rotational perturbations were revealed for the (k − l) = −14 sublevel of ν6 as well as the K = 9 to 16 systems of ν3, the latter mostly being due to Δl = Δk = ±1 and Δl = ±1, Δk = ±2 interactions with ν5. Improved J-dependent ground state constants up to sextic terms have been determined by a fit of 372 combination differences, σ = 7.2 × 10−5 cm−1. An alternative model without ν 3 ν 6 Coriolis x, y resonance has been discarded despite the high correlation of α3B and α6B with ζ3,6." @default.
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- W2040331880 date "1986-09-01" @default.
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- W2040331880 title "High-resolution Fourier transform spectrum and rovibrational analysis of the coriolis coupled ν3 and ν6 fundamentals of H3SiF near 800 cm−1" @default.
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- W2040331880 doi "https://doi.org/10.1016/0022-2852(86)90210-9" @default.
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