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- W2040333821 abstract "The third-order nonlinear optical properties of a polyazine and its oligomers are reported for the first time. Third-harmonic generation measurements revealed a nonresonant third-order nonlinear optical susceptibility χ (3) (-3ω; ω, ω, ω) of 1.53×10 -12 esu for a pentamer and 8.0×10 -12 esu for propylmethylpolyazine at 1.5 µm. Dipole polarizability (α) and second hyperpolarizability (γ) of oligomer model compounds were also calculated by employing the ab initio coupled-perturbed Hartee-Fock (CPHF) theory. Both polarizabilities and χ (3) (-3ω; ω, ω, ω) increase significantly as the length of π-electron delocalization increases in the polyazine backbone." @default.
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- W2040333821 date "1993-02-01" @default.
- W2040333821 modified "2023-09-26" @default.
- W2040333821 title "Studies of Third-Order Nonlinear Optical Properties of Polyazine and Its Oligomers" @default.
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- W2040333821 doi "https://doi.org/10.1143/jjap.32.l193" @default.
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