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• W2040337536 abstract "Measurements of particulate sulfur to total sulfur concentration ratios and 34S-32S isotope ratios were employed to determine the percent of sulfur dioxide converted to sulfate in the plumes of four coal-fired power plants. A fixed-wing airplane was outfitted with a high-volume impregnated filter assembly to collect the samples. A variety of parameters were investigated including relative humidity ranging from 32 to 85%, temperatures from 10 to 25°C, distances as far as 70km and times as long as 200 min. Generally the extent of SO2 oxidation seldom exceeded 5% with essentially all of the observed oxidation occurring within the first few kilometers after emission. The observations are interpreted as indicative of a heterogeneous mechanism with the consumption or poisoning of available catalyst. No distinct correlation was found between the extent of sulfur dioxide conversion with distance, travel time, temperature, relative humidity, time of day or atmospheric stability. Plume reproducibility measurements were made, aircraft flight patterns compared and fringe effects investigated. An extensive body of information has been obtained and should serve as a reference for future investigations." @default.
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• W2040337536 date "1977-01-01" @default.
• W2040337536 modified "2023-09-27" @default.
• W2040337536 title "Further studies on the oxidation of sulfur dioxide in coal-fired power plant plumes" @default.
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• W2040337536 doi "https://doi.org/10.1016/0004-6981(77)90009-9" @default.
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