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- W2040373332 abstract "Solubility data for hydrogen in liquids at low temperature and high pressure have been reduced by a thermodynamic relation similar to the Krichevsky-Kasarnovsky equation but allowing for the variation of activity coefficient with hydrogen concentration. The parameters appearing in this relation have been partially correlated on the basis of a very simple solution model. The results show that under comparable conditions the solubility of hydrogen in simple inorganic solvents (argon, nitrogen and carbon monoxide) is considerably larger than that in light hydrocarbons (ethane, ethylene, propane and propylene), with methane falling in between these groups. On a réduit les données de solubilité de l'hydrogène dans les liquides à basse température et haute pression à l'aide d'une relation thermodynamique analogue à l'équation de Kruchevsky-Kasarnovsky mais permettant de tenir compte des variations du coefficient d'activité avec la concentration en hydrogène. Les paramètres de cette équation ont été corrélés en partie par un modèle très simple de la solution. Il en résulte que dans des conditions comparables la solubilité de l'hydrogène dans les solvants inorganiques (argon, azote et anhydride carbonique) est considérablement plus élévée que dans les hydrocarbures légers (éthane, éthylène, propane et propylène). Le méthane se situe entre ces deux groupes. Löslichkeitsdaten für Wasserstoff in Flüssigkeiten bei tiefen Temperaturen und hohen Drucken sind mittels einer thermodynamischen Beziehung reduziert worden, welche derjenigen von Krichevsky-Kasarnovsky ähnlich ist, aber die Aenderung des Aktivitätskoeffizienten mit der Wasserstoffkonzentration berücksichtigt. Die in dieser Beziehung vorkommenden Parameter konnten zum Teil durch eine Korrelation verknüpft werden, welche auf einem sehr einfachen Lösungsmodell beruht. Die Ergebnisse zeigen, dass unter vergleichbaren Bedingungen die Löslichkeit des Wasserstoffes in einfachen anorganischen Lösungsmitteln (Argon, Stickstoff, Kohlenmonoxid) bedeutend grösser ist als in leichten Kohlenwasserstoffen (Aethan, Aethylen, Propan, Propylen). Methan befindet sich zwischen diesen beiden Gruppen." @default.
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- W2040373332 date "1964-10-01" @default.
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- W2040373332 title "Thermodynamics of hydrogen solubility in cryogenic solvents at high pressures" @default.
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