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• W2040378846 abstract "Infrared—ultraviolet double resonance experiments have been performed to measure total rotational relaxation rates from a single, selected level in C2H2 induced by a variety of collision partners (M). Pulses of tunable infrared radiation from an optical parametric oscillator have been used to excite C2H2 molecules into a rotational level within one or other of the vibrational states arising from Fermi resonance between the zeroth-order 31 and 214151 states. Loss of population from this level was observed by making time-resolved laser-induced fluorescence measurements on the appropriate lines in the A1AuX1Σg+ electronic bands of C2H2. Rate constants are presented for relaxation from the j=12 level of the lower of the Fermi dyads with M=C2H2, He, Ne, Ar, Kr, Xe, H2, N2, O2, CO, NO, HCl, HBr and HCN. A smaller number of results are presented for relaxation from other levels and the data are discussed in the light of energy transfer rates and collision-broadening parameters measured previously for rotational levels in other vibrational states." @default.
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• W2040378846 date "1992-04-01" @default.
• W2040378846 modified "2023-10-06" @default.
• W2040378846 title "Infrared—ultraviolet double resonance measurements on the relaxation of rotational energy in the (31, 214151) Fermi resonance states of C2H2" @default.
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• W2040378846 doi "https://doi.org/10.1016/0009-2614(92)85591-w" @default.
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