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- W2040507368 abstract "Diblock copolymers consisting of poly(N 5-hydroxyalkylglutamine) (PHAG) and poly(N-isopropylacrylamide) (PNIPAAm) were prepared by aminolysis with aminoalkanols of the side-chain ester of poly(γ-benzyl L-glutamate) (PBLG) as a part of PBLG-PNIPAAm block copolymers. The molecular weight ratio of the initial PBLG to the resulting PHAG was nearly 0.35. The effect of PNIPAAm on the conformational change of PHAG in PHAG-PNIPAAm block copolymers with temperature was investigated by circular dichroism. Poly[N 5-(2-hydroxyethyl)-L-glutamine] (PHEG) and the PHEG-PNIPAAm copolymer (GNE) stayed in a randomly coiled conformation whereas poly[N 5-(3-hydroxypropyl)-L-glutamine] (PHPG), poly(N 5-(4-hydroxybutyl)-L-glutamine) (PHBG), PHPG-PNIPAAm copolymer (GNP), and PHBG-PNIPAAm copolymer (GNB) underwent conformational transitions with temperature. The conformational change of the PHPG block in GNP copolymer occurred from an α-helix to a random coil after the incorporation of PNIPAAm into the copolymer. The thermodynamic parameters of the thermally induced helix-coil transition for PHBG and PHBG-PNIPAAm in aqueous solution were calculated." @default.
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- W2040507368 date "2001-02-01" @default.
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- W2040507368 title "Effects of Poly(N-isopropylacrylamide) (PNIPAAm) on the Conformational Change of Poly(N 5-hydroxyalkyl glutamine) (PHAG) in PHAG-PNIPAAm Block Copolymer with Temperature" @default.
- W2040507368 doi "https://doi.org/10.1002/1521-3935(20010201)202:3<395::aid-macp395>3.0.co;2-s" @default.
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