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• W2040519022 abstract "End-functionalized poly(ethylene glycol) (PEG) and polydimethylsiloxane (PDMS) were cross-linked by a thiolene reaction with a tetra-functional thiol to create robust, tunable networks. These networks were loaded with increasing amounts of lithium bis(trifluoromethane sulfonyl imide) (LiTFSI), and their ion conductivity was measured. A wide range of salt loading was achieved, allowing the investigation of both salt-in-polymer and polymer-in-salt regimes. Thermal, mechanical, and ion conductivity properties of LiTFSI-loaded PEG and PEG-PDMS networks were measured. Even at high salt loadings, both networks maintained rubber-like characteristics, which were stable over a range of temperatures (30–90 °C). The PEG network with the highest salt loading showed the greatest ion conductivity, 6.7 × 10–4 S cm–1 at 30 °C, as measured by impedance spectroscopy. This system provides a route to optimize lithium ion conduction and mechanical properties." @default.
• W2040519022 created "2016-06-24" @default.
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• W2040519022 date "2012-05-31" @default.
• W2040519022 modified "2023-10-18" @default.
• W2040519022 title "Tunable Networks from Thiolene Chemistry for Lithium Ion Conduction" @default.
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• W2040519022 doi "https://doi.org/10.1021/mz300090m" @default.
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