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- W2040532465 abstract "Abstract Thermodynamic deuterium substitution effects on reactant conversion and product selectivity were investigated by computer simulation for the stoichiometric partial oxidation of methane. Methane conversion shows a normal deuterium isotope effect, whereas CO selectivity shows an inverse deuterium isotope effect. H 2 selectivity exhibits a large normal deuterium effect. Moreover, deuterium isotope effects are dependent on reaction temperatures and pressures. When reaction pressure is very low, such as 0.001 MPa, all thermodynamic deuterium isotope effects are negligible at 650°C or above. Three criteria, based on the deuterium‐isotope effects, were proposed to determine whether a partial oxidation reaction of methane is kinetically controlled without accurately measured reaction temperatures." @default.
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- W2040532465 date "2003-12-01" @default.
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- W2040532465 title "Thermodynamic isotope effect in partial oxidation of methane to syngas" @default.
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- W2040532465 doi "https://doi.org/10.1002/aic.690491224" @default.
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