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• W2040672610 endingPage "4734" @default.
• W2040672610 startingPage "4719" @default.
• W2040672610 abstract "Quantitative concentration measurements of CH and C2 have been performed in laminar, premixed, flat flames of propene and cyclopentene with varying stoichiometry. A combination of cavity ring-down (CRD) spectroscopy and laser-induced fluorescence (LIF) was used to enable sensitive detection of these species with high spatial resolution. Previously, CH and C2 chemistry had been studied, predominantly in methane flames, to understand potential correlations of their formation and consumption. For flames of larger hydrocarbon fuels, however, quantitative information on these small intermediates is scarce, especially under fuel-rich conditions. Also, the combustion chemistry of C2 in particular has not been studied in detail, and although it has often been observed, its role in potential build-up reactions of higher hydrocarbon species is not well understood. The quantitative measurements performed here are the first to detect both species with good spatial resolution and high sensitivity in the same experiment in flames of C3 and C5 fuels. The experimental profiles were compared with results of combustion modeling to reveal details of the formation and consumption of these important combustion molecules, and the investigation was devoted to assist the further understanding of the role of C2 and of its potential chemical interdependences with CH and other small radicals." @default.
• W2040672610 created "2016-06-24" @default.
• W2040672610 creator A5036966643 @default.
• W2040672610 creator A5046072802 @default.
• W2040672610 creator A5049514549 @default.
• W2040672610 creator A5069149845 @default.
• W2040672610 date "2010-02-05" @default.
• W2040672610 modified "2023-10-10" @default.
• W2040672610 title "Quantitative Laser Diagnostic and Modeling Study of C₂ and CH Chemistry in Combustion" @default.
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• W2040672610 doi "https://doi.org/10.1021/jp908242y" @default.
• W2040672610 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/20136115" @default.
• W2040672610 hasPublicationYear "2010" @default.
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