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• W2040783062 abstract "Infrared optical spectra have been investigated for a charge-transfer complex of tetrathiafulvalene and 2-bromo-3,5,6-trichloro- $p$-benzoquinone, which undergoes a neutral-ionic ( $Nensuremath{-}I$) transition at ${T}_{c}phantom{rule{0ex}{0ex}}=phantom{rule{0ex}{0ex}}68mathrm{K}$. With the decrease of temperature toward ${T}_{c}$, the far-infrared reflectivity spectrum is gradually transformed into a Drude-like high reflectance band edging around $100{mathrm{cm}}^{ensuremath{-}1}$, and the optical conductivity shows an anomalous peak around $10{mathrm{cm}}^{ensuremath{-}1}$. The far-infrared anomaly is related to the gigantic dielectric response just above ${T}_{c}$, which are both discussed in terms of dynamics of $Nensuremath{-}I$ domain walls with fractional charge." @default.
• W2040783062 created "2016-06-24" @default.
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• W2040783062 date "2001-10-11" @default.
• W2040783062 modified "2023-10-04" @default.
• W2040783062 title "Far-Infrared Optical Response of Neutral-Ionic Phase Transition in an Organic Charge-Transfer Complex" @default.
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• W2040783062 doi "https://doi.org/10.1103/physrevlett.87.187401" @default.
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